[HN Gopher] Low-Temperature Additive Manufacturing of Glass
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       Low-Temperature Additive Manufacturing of Glass
        
       Author : LorenDB
       Score  : 97 points
       Date   : 2025-06-18 16:13 UTC (4 days ago)
        
 (HTM) web link (www.ll.mit.edu)
 (TXT) w3m dump (www.ll.mit.edu)
        
       | jiehong wrote:
       | Very cool indeed!
        
       | giantg2 wrote:
       | Interesting. I wonder if this could be used to print telescope
       | mirrors if you could get an "ink" that has high thermal
       | stability, or if that would be in conflict with the low
       | temperature printing.
        
         | hbrav wrote:
         | That seems like it would be very difficult. For a telescope
         | mirror you want a very good surface finish, and that's one
         | thing that 3D printing does very poorly.
        
           | giantg2 wrote:
           | The polishing process could be done differently. If you could
           | print the specific parabolic shape, that could save a lot of
           | time hogging out. Although slumping might work better if
           | surface ends up smoother. Im not sure of the annealing
           | process might go.
        
             | taneq wrote:
             | There's a few combined-process setups coming out these days
             | that use 3D printing as a first pass and then machine the
             | print in-place before sintering etc. which saves a ton of
             | setup and fixturing time.
        
               | sheepscreek wrote:
               | Yes! This is exactly what I had in mind. Sintering
               | (thanks for the term) combined with this 3D printing
               | technique could still make the process faster and lead to
               | more consistent results.
               | 
               | Now that's I think about it, one could in theory use the
               | exact same process for plastic-polymer lenses too, albeit
               | at lower temperatures (better).
        
             | bhickey wrote:
             | The parabola of a telescope mirror generally deviates from
             | a sphere by tens of micrometers at best. Figuring happens
             | after grinding and after polishing. Slumping is neat, but
             | I've heard from the grognards that they can shatter if the
             | temperature changes too quickly.
        
         | sheepscreek wrote:
         | Maybe with further augmentation to the process. The 3D printing
         | seems to leave pretty big grooves on the glass - which can
         | distort the passage of light. For any real optical application,
         | that will have to be removed somehow. Such as baking the glass
         | structure in a high heat oven with a centrifuge/fast spinning
         | base and some kind of mould to put the initial piece on.
         | 
         | The high heat and spin action could, in theory, fuse the
         | individual grooves for a more uniform dispersion of light, and
         | the mould shape would further press on the glass to maintain or
         | alter its shape to be closer to a lens.
         | 
         | Finish that off with fine "sanding" and/or polish, and that
         | might do the trick?
         | 
         | Honestly, experimentation might be the only way to find out.
        
         | kragen wrote:
         | You'll probably be interested in
         | https://dercuano.github.io/notes/gradient-refractive-
         | index.h..., which isn't exactly what you described.
        
       | metalman wrote:
       | this is a highly missleading "anouncement" about sodium silicate
       | "glass"(ish),stuff
       | 
       | https://en.wikipedia.org/wiki/Water_glass
       | 
       | but if you want to plqy with some, it is readily avail8ble as a
       | "cement" used for attaching seals to wood stove doors, and
       | countless other low teck applications the comon name of "water
       | glass" refers to it's solubility, so.....
        
         | bahmboo wrote:
         | That's not what this is. Sodium silicate is part of the process
         | but so are lots of other things. The patent is posted here in
         | the comments that would be a good place to start if one wanted
         | to experiment with it.
        
       | gsf_emergency_2 wrote:
       | https://patents.google.com/patent/US11499234B2/en
       | 
       | I wonder what the other inorganics ("functional additive,
       | embodied in some cases by Silver flakes") are, exactly. In their
       | flagship product.
       | 
       | And the size of the nozzle, why not the easier to remember 400
       | micrometers?
        
         | ricardobeat wrote:
         | What do you mean about the nozzle? They describe it in microns:
         | 
         | > The ink can be extruded through a nozzle 604 (e.g., a 200 mm,
         | luer-lock tapered nozzle)
        
       | kragen wrote:
       | So it sounds like a single-component process, no powder bed or
       | vat of hardener liquid. "Silicate solution" presumably means
       | waterglass rather than something like tetraethyl orthosilicate,
       | and if it hardens rather than foaming up at 250deg, it's either
       | because they're doing the process under pressure or, more likely,
       | the other inorganics they mention are donating polyvalent cations
       | such as Ca++, Mg++, Al3+, or Fe3+ to crosslink the silicate
       | residues.
       | 
       | Probably the polyvalent cations are bound up in a salt that has
       | negligible solubility at room temperature, so the ink doesn't
       | harden in the reservoir, but which can react with the silicate at
       | 250deg, maybe a hydroxide or carbonate. Calcium sulfate is
       | probably too soluble.
       | 
       | Presumably the silica filler is amorphous and serves to
       | strengthen the glass and reduce the TCE, though it probably
       | raises the cost. Maybe it also makes the paste thixotropic
       | without needing to include organics like carboxymethylcellulose
       | which would be hard to remove later. And I guess maybe it could
       | react directly with the waterglass to solidify it, in effect
       | raising the waterglass's modulus out of the water-soluble region,
       | without requiring any polyvalent cations. Silica fume is the most
       | likely form of silica here.
       | 
       | If anyone digs up more details, I'd love to see them.
       | 
       | Hmm, I see gsf_emergency_2 found this patent from 02020:
       | https://patents.google.com/patent/US11499234B2/en which is later
       | than Dercuano but earlier than Derctuo and Dernocua. But its
       | priority date is from a provisional patent application from
       | 02019, so even Dercuano doesn't count as prior art, even if it
       | anticipates some of the claims. Also, though, I don't see
       | anything that anticipates this process in notes like
       | https://dercuano.github.io/notes/flux-deposition.html and
       | https://dercuano.github.io/notes/powder-bed-3d-printing.html,
       | which suggests that it wasn't as obvious as it sounds.
       | 
       | The patent says, "curing the material to evolve gaseous water,"
       | which makes it sound like thick sections _would_ foam up. (You
       | have to heat it over a length of time quadratic in section
       | thickness to permit water to diffuse through the nascent solid.)
       | And supposedly that is the purpose of the heating, rather than
       | provoking the other reactions I speculated about above.
       | 
       | There are some interesting notes in the patent about promising
       | functional fillers, such as carbon fiber for strength or silver
       | flakes or conductivity. It suggests using these inert fillers at
       | loadings of 45% to 90%.
       | 
       | It confirms that the silica is fumed silica, and suggests as
       | alternatives fumed alumina (sapphire) or fumed titania (rutile or
       | anatase), which are not products I had heard of, though titania
       | nanoparticles are common as a white pigment in paint and in food.
       | Waterglass can definitely crosslink with aluminate sources such
       | as metakaolin, as used in "geopolymer cement". Titanate is news
       | to me, if true.
       | 
       | It also confirms my inference that the fumed silica makes the ink
       | thixotropic, at 15 wt%, though it uses the phrasing, "introduces
       | a yield stress into the material" and "shear-thinning behavior".
       | 
       | I'm definitely going to use that phrase the next time I'm making
       | mayonnaise.
       | 
       | "Why are you stirring that bowl of egg yolks and oil with a
       | fork?"
       | 
       | "I'm introducing a yield stress into the material!"
       | 
       | The patent also confirms my inference that the silicate solution
       | is waterglass; it specifically says sodium silicate (or ammonium
       | silicate, which is probably not a practical possibility:
       | http://www.sciencemadness.org/talk/viewthread.php?tid=10297)
       | 
       | The patent doesn't suggest using ionotropic gelation in the way I
       | suggested at all. It doesn't mention the mineral oil either.
        
         | MonkeyClub wrote:
         | > from 02020
         | 
         | Is the year in octal (/s), or do you truly believe we're due to
         | survive eight more millennia with the same year numbering
         | system?
        
           | nemomarx wrote:
           | I think the long now foundation tries to promote it to raise
           | awareness and get people thinking about the future
           | consequences of things.
           | 
           | It seems very optimistic and 90s to me now
        
           | jagged-chisel wrote:
           | https://news.ycombinator.com/item?id=43613664
        
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