[HN Gopher] Newly discovered deep-sea enzyme breaks down PET pla...
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       Newly discovered deep-sea enzyme breaks down PET plastic
        
       Author : hanniabu
       Score  : 145 points
       Date   : 2023-09-26 13:52 UTC (9 hours ago)
        
 (HTM) web link (phys.org)
 (TXT) w3m dump (phys.org)
        
       | dzdt wrote:
       | The way to understand the origin of fossil fuel deposits is that
       | hundreds of millions of years ago trees were made of plastic.
       | 
       | Thats not quite literally true but it gives the right sense. In
       | the Carboniferous period trees grew abundently but there were not
       | yet bacteria that could break down the lignins composing the
       | woody structure. Its very similar to what you'd get with plastic
       | trees today: they would fall and pile up like junk in a landfill.
       | Then eventually this would be buried and result in the many-
       | meters-thick coal deposits we find today.
       | 
       | Lessons? I don't know. But piles of un-decomposable hydrocarbons
       | is not a new thing for the planet.
        
         | morsch wrote:
         | When I searched for this, I found there to be some debate on it
         | (isn't there always?):
         | https://www.pnas.org/doi/10.1073/pnas.1517943113
         | https://arstechnica.com/science/2016/01/why-was-most-of-the-...
        
           | dzdt wrote:
           | Thanks! Your newer research is pretty convincing. Makes me a
           | bit sad: I really like the 'plastic tree' analogy. Ah, well.
        
         | bno1 wrote:
         | I wonder what forests looked back then. Trees going through and
         | on piles of dead trees?
        
         | m463 wrote:
         | It's interesting to read about thomas gold's theories about
         | hydrocarbons.
         | 
         | https://en.wikipedia.org/wiki/Abiogenic_petroleum_origin
         | 
         | To me it makes sense that some or all hydrocarbons are or at
         | least started like the hydrocarbons found on other planets in
         | our solar system.
        
       | zellyn wrote:
       | I love the idea of finding enzymes that break down plastics. I
       | also like to imagine the post-apocalyptic Sci-Fi short story
       | possibilities of accidentally releasing something that breaks
       | down _all_ plastic!
       | 
       | Imagine my delight in reading this:                   At the
       | molecular level, PET46 is very similar to another enzyme, ferulic
       | acid esterase. This degrades the natural polymer lignin in plant
       | cell walls         by breaking down lignin polymers to release
       | sugars from woody plant parts.         Lignin and PET have many
       | structural similarities, so the PET-degrading         enzymes
       | found in nature may be important for composting wood in forest
       | soils, for example.
       | 
       | Now, join me in imagining the post-apocalyptic Sci-Fi short story
       | possibilities of accidentally releasing something that breaks
       | down all plastic _and_ all plants! I mean, until some of them
       | finally adapt.
        
         | lanstin wrote:
         | Unlike the plastic substrate of modern technological society,
         | plants have survived hundreds of millions of years of efforts
         | by the rest of the biosphere to eat them.
        
           | zellyn wrote:
           | True, although I believe dredging up unusual enzymes from the
           | stygian depths facilitates new and exciting dystopian
           | storylines.
        
             | aftbit wrote:
             | You might enjoy the Rifters trilogy by Peter Watts.
        
       | multiplegeorges wrote:
       | So dumping all our plastic in the sea will work out! /s
       | 
       | It seems like these discoveries are coming quickly and in higher
       | numbers. Maybe there's hope in recycling/processing plastics down
       | simpler molecules after all. Currently, recycling plastic is a
       | bit of a lie -- very little of it is actually recycled.
        
         | titzer wrote:
         | I recognize the sarcasm in your first sentence, but I am not
         | super hopeful. The question is always, "so now it breaks
         | down...into what? And what happens to that?". If that gives
         | rise to the equivalent of some kind of algal bloom that then
         | kills off other life, it might actually be worse than the
         | microplastics themselves.
         | 
         | I for one do not hold out hope for recycling plastics. We had
         | more sustainable materials in the past, and in places we still
         | do that. For example, reusing beer bottles with the Pfand
         | system in Germany, or milk bottles, crates, durable packaging.
         | We're still going backwards with this consumerist throwaway
         | culture.
        
           | EGreg wrote:
           | Here here.
           | 
           | Unfortunately the government has teamed up with the
           | corporations to continue to push it for decades:
           | 
           | https://magarshak.com/blog/?p=362
           | 
           | The recycling was a scam to keep the public distracted so
           | their impulse to "do something" would lead to individuan
           | action rather than lead to organizing to demand reforms!
        
         | kzrdude wrote:
         | I'm fearing that degradable plastics is also a lie.. is it just
         | turning it into microplastics small enough that the problem
         | visually disappears?
        
           | Kerb_ wrote:
           | It breaks them down into their atomic components and enables
           | bacteria that can straight up digest plastic. The issue from
           | this is that we rely on plastics not being degradable for a
           | lot of the properties we use it for. Imagine if bugs got this
           | enzyme in their gut bacteria, and started eating the food
           | wrappers instead of just nibbling through them. Plastic used
           | to seal sterile equipment in medical settings or for
           | implants? Useless. The plastic waste would only last a few
           | years relative to the decades+ now, but it would also ruin
           | plastic's ability to seal stuff, which is why we use it.
           | 
           | Overall, probably a good thing to reduce our reliance on
           | plastic, but it will come at a cost, it's not just "we can
           | dump plastic in the ocean now"
        
             | coffeebeqn wrote:
             | It would still be difficult for bugs to gnaw on solid
             | plastic
        
         | hutzlibu wrote:
         | "Currently, recycling plastic is a bit of a lie -- very little
         | of it is actually recycled."
         | 
         | Depends where you live and what you consider recycling. If you
         | mean, making new plastics out of the old, than the challenge
         | is, that there are many, many different plastics you cannot
         | just melt in and reuse if mixed together. A annoying, but
         | working solution here in germany is a mandated bottle bill.
         | Meaning you pay 25 cent extra per bottle, and get it back, if
         | you return that bottle into a machine: but this results in
         | actual reusable plastics as they are all of the same kind.
         | 
         | And for the rest, the most pragmatic solution is burning it for
         | energy. If you use filters, it is not so bad and it is
         | recycling, but it is the same as burning fossil fuels, so not a
         | good long term solution.
        
           | gruez wrote:
           | >And for the rest, the most pragmatic solution is burning it
           | for energy.
           | 
           | No, burying is better because it sequesters the carbon rather
           | than releasing it into the atmosphere.
        
             | hutzlibu wrote:
             | If it means not burning coal, oil or gas instead and there
             | are good filters, I think burning plastic makes sense. But
             | if you can actually get all the needed energy from non
             | fossil sources, then yes, burying makes more sense. But I
             | think only some rare places on earth are that far.
        
           | digging wrote:
           | > And for the rest, the most pragmatic solution is burning it
           | for energy.
           | 
           | I really wish we'd do more of this. I know it's not ideal,
           | but we in the US need to treat plastic like the trash that it
           | (mostly) is. And trash is just fuel. Instead we have
           | convenient single-stream recycling which means all our actual
           | recyclables also end up in the trash and/or oceans.
        
             | ZeWaka wrote:
             | We actually do a fair amount of this in the US. Marion
             | County in Oregon burns 90% of their trash. It's much better
             | than landfills, anyways.
        
               | gruez wrote:
               | How is burning better than landfilling it? If the
               | landfill is lined the garbage isn't going anywhere, and
               | leaving the plastic in the ground is much better than
               | releasing its co2 into the atmosphere. Land use might be
               | an issue in some places, but I doubt that's the case in
               | Oregon.
        
       | kwhitefoot wrote:
       | Why do we want to break down PET? Why not just re-use it?
        
         | Intralexical wrote:
         | Heat, stress, and light will probably break it down
         | mechanically over time no matter how diligent you are about
         | reusing or recycling it.
         | 
         | At the very least, this should hopefully mean that all those
         | scary endocrine-disrupting and bioaccumulating microplastic and
         | nanoplastic particles that are apparently being shed by the
         | millions every time you heat or handle anything plastic aren't
         | necessarily going to keep building up forever.
        
         | wahnfrieden wrote:
         | Most is not reused, or only reused with limited capacity
        
       | ginko wrote:
       | Now splice this into the genome of black mold and release it in a
       | coca-cola bottling plant.
        
         | tabtab wrote:
         | Don't laugh, someday a terrorist or hacker may engineer a fast-
         | eating critter, and half our stuff will become useless in a
         | year. Termites learned to work with gut microbes to speed up
         | wood munching, a home-owner's biggest nightmare.
        
           | izzydata wrote:
           | That's still kind of funny in a existential hysteria kind of
           | way.
        
           | hansvm wrote:
           | Humans are pretty adaptable. If half our stuff did become
           | useless do you think that might put a damper on rampant
           | consumerism?
        
             | hanniabu wrote:
             | It would increase consumerism since everything would need
             | to be replaced on a periodic basis
        
               | digging wrote:
               | Everything? I think instead, we'll just stop making most
               | things out of plastics. We have longer-lasting, more
               | durable materials than plastics already, for when you
               | want something that will actually survive decades or
               | generations. They're metals and woods and stones.
               | 
               | Some things, like wire coatings, will still likely need
               | to be plastic and will become disposable. But most uses
               | of plastic for long-lasting goods will just stop using
               | plastics. Goods will get much heavier, but more durable.
        
               | ars wrote:
               | Woods? If wood can survive so can plastic in this
               | hypothetical world. Just keep water away from the
               | plastic.
        
               | BizarroLand wrote:
               | With new plastics full of chemicals that the bugs won't
               | eat.
        
         | Metacelsus wrote:
         | Sounds like "Mutant 59"
        
         | monocasa wrote:
         | Less fun, PET is heavily used in medical devices including
         | implants. There's a huge cut to life expectancy if it becomes a
         | secondary food source for something like an engineered MSRA
         | strain.
        
           | digging wrote:
           | More reason to be furious at plastic peddling billionaires.
           | They made us hostages. We still have to stop them, but it's
           | going to hurt even more.
        
             | Intralexical wrote:
             | Eh. Thinking plastic would last forever was probably a
             | reasonable assumption at the time. I doubt it was the
             | billionaires making that design call. Though in hindsight
             | maybe we should have known better, given the history of
             | lignin and natural waxes.
             | 
             | Though especially given the history of lignin, we probably
             | have millions of years before medical devices being eaten
             | by microbes becomes a widespread problem that anyone
             | seriously needs to worry about. There's bigger fish to fry
             | right now.
        
               | digging wrote:
               | > Thinking plastic would last forever was probably a
               | reasonable assumption at the time
               | 
               | That's... not what I'm mad about at all.
        
         | [deleted]
        
         | walnutclosefarm wrote:
         | The Andromeda Strain!
        
           | mattkrause wrote:
           | Or Peter Watts' _Starfish_ , since it's from the deep sea
        
             | digging wrote:
             | There's one significant detail about Behemoth missing...
        
       | rand0mx1 wrote:
       | AMP-Free link
       | 
       | https://phys.org/news/2023-09-newly-deep-sea-enzyme-pet-plas...
        
         | dang wrote:
         | Changed from https://phys.org/news/2023-09-newly-deep-sea-
         | enzyme-pet-plas.... Thanks!
        
       | sproketboy wrote:
       | [dead]
        
       | perlgeek wrote:
       | Thank you phys.org for putting an actual link to the scientific
       | publication, something that is missing far too often these days.
        
       | gilleain wrote:
       | Slightly misleading headline, as PET (polyethylene terephthalate)
       | hydrolases were already known - see
       | https://www.chm.bris.ac.uk/motm/PETase/PETaseh.htm
       | 
       | This is a study of an archaeal enzyme (from the deep-sea) that
       | can degrade both long-chain and short-chain polymers that is more
       | efficient at 70 deg C than other enzymes.
       | 
       | The details are that this is a feruloyl esterase with a conserved
       | alpha/beta-hydrolase fold but with an additional flexible 'lid'
       | domain that covers the active site. The authors suggest this lid
       | domain replaces the conserved Trp that is an Ala in the archaeal
       | enzyme.
        
         | hanniabu wrote:
         | > Slightly misleading headline, as PET (polyethylene
         | terephthalate) hydrolases were already known
         | 
         | It doesn't say it was the only one, just a newly discovered one
        
           | gilleain wrote:
           | Sure, fair enough. I just thought people might read it as
           | "Enzyme with new ability (to break down PET) discovered", but
           | maybe I was being pessimistic.
        
             | capableweb wrote:
             | It's also mentioned in the article body:
             | 
             | > Until now, about 80 different PET-degrading enzymes were
             | known, most of which were found in bacteria or fungi.
        
               | digging wrote:
               | Most of us aren't reading the body though.
        
         | pneumic wrote:
         | Yeah, it's not bad news at all but it appears to be one of many
         | that still require considerable heat, industrial infra, etc.
         | 
         | Has anyone attempted to put these enzymes to the test in at
         | some scale in an industrial setting, I wonder?
        
           | hanniabu wrote:
           | Should work well in landfills since there's heat buildup
        
           | jamesjuicy55 wrote:
           | https://www.purecycle.com/who-we-are. ?
        
           | hinkley wrote:
           | I mean my processor hits 70deg and has for a decade or more,
           | and my car engine thinks 87deg is the happy temperature.
           | 
           | 70deg is maybe a little out of the reach of a home system but
           | nothing for a municipal system. Right?
        
           | gilleain wrote:
           | No idea. From skimming some university press releases, I see
           | a lot of "potential for!" and similar wording.
           | 
           | This https://news.utexas.edu/2022/04/27/plastic-eating-
           | enzyme-cou... has "Up next, the team plans to work on scaling
           | up enzyme production to prepare for industrial and
           | environmental application. " which is more promising.
           | 
           | As far as I understand, yes it is a very different challenge
           | to make a bioreactor for actually using some random new
           | enzyme than the (also hard) problem of getting the structure
           | in the first place. How to immobilize it on some surface, how
           | to pre-process the material to pass it through the reactor
           | (?) I guess ...
        
             | justaskme wrote:
             | Feels like it's always "potential for"... _sigh_
        
           | eindiran wrote:
           | I was recently at a party and spent some time talking with
           | someone who has a stealth startup working on this exact
           | problem. He said that they aren't the first, but getting the
           | scale right (in an industrial setting) and finances right
           | enough that someone is willing to spend the money to set it
           | up is far harder than just finding an enzyme that can break
           | down PET / similar polymers.
        
         | testfoobar wrote:
         | "this is a feruloyl esterase with a conserved alpha/beta-
         | hydrolase fold but with an additional flexible 'lid' domain
         | that covers the active site"
         | 
         | As educated as I think I am, it is always humbling to read a
         | hacker news comment that I cannot understand.
         | 
         | ELI5?
        
           | gilleain wrote:
           | Apologies, that was meant for the specialists :) It is mostly
           | just technical jargon so do not feel too humble ...
           | 
           | So I'll break it down:
           | 
           | - "feruloyl esterase" : an 'esterase' is an enzyme that makes
           | or breaks ester bonds. In this case, 'feruloyl' which I've
           | never heard of but apparently is some small molecule that is
           | normally attached to a sugar.
           | https://en.wikipedia.org/wiki/Feruloyl_esterase
           | 
           | - "conserved alpha/beta-hydrolase fold" : a structural
           | pattern (fold) that is shared (conserved) between a set of
           | structures. In other words, these enzymes all have roughly
           | the same shape. https://www.cathdb.info/version/v4_3_0/superf
           | amily/3.40.50.1...
           | 
           | - "additional flexible 'lid' domain that covers the active
           | site" : a 'domain' is just a compact part of a protein,
           | without going into too much detail. They are calling it a
           | 'flexible lid' as the idea is that it moves out of the way to
           | bind the substrate to the active site (where the reaction is
           | carried out) and back again when fully bound.
        
             | testfoobar wrote:
             | Thank you.
        
           | neftaly wrote:
           | Enzymes are kind of like a tool for breaking apart lego
           | blocks, or a jig for assembling them. This sounds like a
           | moving part that covers the "teeth" and makes it more
           | effective (or less likely to get jammed by the wrong
           | molecules?).
        
             | Gibbon1 wrote:
             | Two things.
             | 
             | Lot of reactions are energetically favorable. But the
             | reactants are stuck in a local minima. So either doesn't
             | happen or is too slow. Enzymes mediate the reaction so it
             | can happen or happen faster.
             | 
             | Lot of reactions there are side reactions that produce
             | stuff you don't want. Resulting a terrible yield or maybe
             | none. Enzymes can promote the reaction you want increasing
             | the yield.
             | 
             | Interesting thing to watch for is eletrocatalysts. Where
             | you use electricity and a catalist to push a reaction that
             | is energetically unfavorable. Like CO2 + H2O --> methanol.
             | These may become very important as we stop pumping oil and
             | gas out of the ground.
        
           | anon84873628 wrote:
           | I don't think there's much to say besides "slightly different
           | chemical structure makes it better". At some point you hit
           | jargon rock bottom.
        
       | FredPret wrote:
       | It's really awesome that all our plastic will one day rot.
       | 
       | But we have lots of pipes and cables underground that will need
       | to be replaced - with what I wonder.
        
       | Max-q wrote:
       | As much plastic as we dump into nature now, we increase the
       | chance for a mutation of a microbe being able to digest it.
       | 
       | If that microbe manage to multiply and spread, plastic can start
       | to rot, just like wood is doing now. On a long term basis, that
       | might be a good thing, but in the short term it would be a
       | catastrophy. We are using plastic as a long lasting material,
       | often with no surface treatment. Imagine if wire insulation,
       | waterproof encapsulation, gaskets and other important parts of
       | our infrastructure starts to rapidly degrade!
       | 
       | That alone should be motivation for cleaning up and stop
       | spreading plastic waste in nature.
        
         | geoelectric wrote:
         | IIRC, "plastic eater" was one of the mutations of The Andromeda
         | Strain in the eponymous Crichton novel.
        
         | vagab0nd wrote:
         | Not to undermine your point about cleaning up plastic, but
         | following your logic: isn't this similar to the antibiotics
         | situation, just maybe on a longer time scale? The more you use
         | it the less effective it is. What's the ultimate solution?
        
           | yukkuri wrote:
           | Walls and ladders. There isn't a solution to evolution, you
           | just have to keep adapting.
        
             | Intralexical wrote:
             | Is it feasible for something like, e.g., teflon to be
             | decomposed biologically?
        
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