[HN Gopher] A Baking Soda Solution for Clean Hydrogen Storage
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       A Baking Soda Solution for Clean Hydrogen Storage
        
       Author : geox
       Score  : 26 points
       Date   : 2023-06-12 23:04 UTC (23 hours ago)
        
 (HTM) web link (www.pnnl.gov)
 (TXT) w3m dump (www.pnnl.gov)
        
       | photochemsyn wrote:
       | Hydrogen is needed for all kinds of industrial processes, but it
       | is best generated at the point of use as needed, as storage and
       | transport is too problematic. If absoultely needed, the most
       | obvious way to ship hydrogen is as methane.
       | 
       | Synthesis of methane from water-sourced hydrogen and atmosphere-
       | sourced CO2 is at present a good deal more expensive than fossil
       | natural gas, but that's a somewhat artificial situation: natural
       | gas production is heavily subsidized and many of the costs are
       | externalized to the public (see global warming, air and water
       | pollution, etc.). However, once accomplished you can just feed
       | this renewable methane into the existing natural gas
       | infrastructure, and get the hydrogen back as needed from well-
       | understood processes, i.e. steam-methane reforming.
        
         | hannob wrote:
         | > If absoultely needed, the most obvious way to ship hydrogen
         | is as methane.
         | 
         | Methane has 2 problems: 1. it's a massive greenhouse gas if it
         | leaks, 2. it requires CO2 to make, and in a decarbonized future
         | that can only come from either biomass (limited) or DAC
         | (expensive).
         | 
         | You would either want ammonia or methanol. Ammonia does not
         | have any of these problems, but it's very toxic. Methanol has
         | the CO2 problem as well, but it's a liquid, so it's easier to
         | transport. Neither is perfect, but there are no perfect
         | solutions.
         | 
         | Methane is the worst of all options. If you want a hydrocarbon,
         | then usually methanol is what you want. And don't trust me on
         | that, just look at what projects are actually planned out
         | there. Plenty of green ammonia and green methanol projects,
         | green methane is exotic at best, barely anyone wants to do
         | that.
        
           | marcosdumay wrote:
           | > Ammonia does not have any of these problems
           | 
           | Ammonia is a greenhouse gas itself, and it tends to react
           | with air creating various nitrous oxides, that are much more
           | potent greenhouse gases than methane, very toxic, and create
           | acid rain (after what it becomes fertilizer).
           | 
           | The best shipping option is probably just to face all the
           | issues and ship the hydrogen. But storage is a different
           | matter.
        
             | hannob wrote:
             | Ammonia is no greenhouse gas, it has a GWP of zero. Burning
             | ammonia produces N2O, which is a potent greenhouse gas, and
             | NOx, which is an air pollutant. But these can be taken care
             | of by scrubbers, and are irrelevant if you ship ammonia for
             | other uses. (I mean the biggest use case of hydrogen these
             | days is making ammonia for fertilizers.)
        
           | photochemsyn wrote:
           | It's not a greenhouse gas if you make it from atmospheric
           | CO2, that's the whole point. Also, sending methane through a
           | pipeline is pretty straightforward. Methanol is an option on
           | the liquid side, but if you can make methanol from
           | atmospheric CO2 and water, you can also make jet fuel, which
           | will be needed as jet travel isn't really electrifiable.
        
       | bagels wrote:
       | "In a renewable energy grid, batteries can handle about 80
       | percent of storage needs."
       | 
       | Why couldn't you just add 25% more batteries?
        
         | ZeroGravitas wrote:
         | Most storage is short term, so the same battery can be re-used
         | again and again by charging and discharging it, e.g. 365 solar
         | peaks a year in sunny countries. Longer term storage would lock
         | up the battery for longer, which given the cost of batteries,
         | wouldn't make financial sense.
        
         | marcosdumay wrote:
         | It's not 25% more batteries. It's some 500% to 1000% more. But
         | those would be used very few times.
        
           | chrisco255 wrote:
           | So in other words batteries don't get us anywhere close to
           | 80% of the way.
        
             | elcritch wrote:
             | Depends on how you're slicing it. By the total flux of
             | energy batteries may be able to handle 80% of the "energy
             | traffic" over the course of a day by smoothing out
             | day/night cycles.
             | 
             | However that last 25% needs to be stored over long periods
             | where the cost is prohibitive to store in current battery
             | systems.
        
             | audunw wrote:
             | There's many ways to judge what "80%" is. The batteries
             | will cycle many times every week. They will have much more
             | energy flowing through them in a year than the storage we
             | need for dunkelflaute would.
             | 
             | Yes, in terms of amount of energy stored at full capacity,
             | batteries would not get us to 80%. But those last 20% have
             | reduced requirements for charge/discharge rates, effiency,
             | cost/kWh, which makes many other solutions viable.
        
       | scythe wrote:
       | This is remarkably hard to follow. The actual technology at play
       | here is bicarbonate-formate redox; as the linked paper states:
       | 
       | >It is also clear that more integration between the disciplines
       | of electrochemistry and heterogeneous catalysis is needed to
       | overcome the challenges for advancing the HCO3--HCO2- system as a
       | feasible green alternative for storing and transporting energy.
       | 
       | The idea of storing energy by converting bicarbonate to formate
       | has already occurred to me years ago and probably was thought of
       | by thousands of other scientists, because formate is one of the
       | most common hydrogen precursors used in practical chemistry. The
       | storage density is low, but the materials are extremely cheap and
       | stable. Unfortunately, the paper does not seem to be announcing a
       | breakthrough, but tallying up the current progress -- which just
       | isn't there yet.
       | 
       | https://pubs.rsc.org/en/content/articlelanding/2023/gc/d3gc0...
        
         | elcritch wrote:
         | Thanks for linking the real article. It's an interesting read,
         | especially that the Gibb's Free Energy for formate-bicarbonate
         | is so low. Ammonia is about 20-40x higher!
         | 
         | Looks like they're using Pd/Pt for the best catalyzers...
         | that's definitely not going to be scalable. Though there should
         | be effective alternatives, but it's surprising how
         | unsophisticated much of the research in this field can be.
        
         | chrisco255 wrote:
         | The article wastes so much time on cutesy fluff. It's almost
         | always a tell that the story is a non-story.
        
         | jfengel wrote:
         | I suppose... a "hydrogen battery" for solar? Build up formate
         | (in solution? As a salt?) during the day, then burn it at night
         | for electricity?
        
           | rfgmendoza wrote:
           | density is not really a critical factor for grid level or
           | onsite energy storage, so it could be feasible in theory
        
             | elcritch wrote:
             | As long as the electrodes / membranes for the conversion to
             | electricity are stable and cheap as well. There's a big
             | downside with PEM electrodes requiring platinum and with
             | their longevity and energy density relative to capex.
        
       | wilg wrote:
       | [flagged]
        
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