[HN Gopher] Atomic resolution video of salt crystals forming in ...
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       Atomic resolution video of salt crystals forming in real time
        
       Author : rbanffy
       Score  : 330 points
       Date   : 2021-01-22 18:28 UTC (4 hours ago)
        
 (HTM) web link (www.u-tokyo.ac.jp)
 (TXT) w3m dump (www.u-tokyo.ac.jp)
        
       | zaroth wrote:
       | Truly mind blowing being able to actually see the atoms align in
       | an instant and the crystal structure just pop into existence.
       | 
       | Hard to believe it's not a computer model. I mean, I guess
       | underneath there must be a hell of a lot of signal processing
       | going on to render that video, but atomic-scale video is wild.
       | 
       | Funny that it looks kinda like MPEGS online circa 1990s.
        
         | mywittyname wrote:
         | I also love how you can see the probabilistic nature of
         | electron orbitals in action. The crystal fades in and out of
         | existence during the early stages of nucleation. And even after
         | the structure is established, the boundaries continue to be
         | "fuzzy."
         | 
         | Even the movement of the crystal looks like a wave, but I don't
         | know if that's because matter moves as a wave at the atomic
         | level or if that's just an artifact from the camera.
        
           | jng wrote:
           | I would think that the coming in and out of view at the
           | beginning is more related to the crystal moving around and
           | falling "in and out of focus" (whatever that means for this
           | type of camera). I'd love to watch quantum probability wave
           | fluctuations, but I think we're still pretty far from probing
           | that.
        
             | jtaillon wrote:
             | In this case, "in and out of focus" is actually variations
             | in the amplitude of the probability function for the
             | electron density projected onto a single plane (to a first
             | approximation). Sometimes the wave functions of all the
             | electrons interfere constructively, so you see a bright
             | spot, and sometimes deconstructively, so you see dark.
             | Depending on the orientation of things, this results in the
             | images of "atoms" that you see in the picture. As the
             | crystal changes shape and size, the interference patterns
             | change, which partially explains why it disappears and
             | reappears a few times. There's a bit more going on than
             | that, but the physics of what's happening in a TEM image is
             | really neat.
        
               | jng wrote:
               | Wow, mind blown. Thanks for correcting me. Amazing to
               | learn that the wave function is so directly sampled by
               | TEM that the image we get shows Moire patterns caused by
               | its phase :)
        
           | Osmium wrote:
           | > I don't know if that's because matter moves as a wave at
           | the atomic level or if that's just an artifact from the
           | camera.
           | 
           | Artifact of the imaging, note the time scale of the movie,
           | it's much longer than any quantum oscillation. Each
           | individual image of the movie is taken eons apart from the
           | perspective of the crystal.
        
             | magicalhippo wrote:
             | > Each individual image of the movie is taken eons apart
             | from the perspective of the crystal.
             | 
             | Given the timescales of atomic reactions, which IIRC is
             | typically measured in nano- or picoseconds, this video is
             | more like watching galaxies form I suppose.
        
       | kvakkefly wrote:
       | You may also like my paper " Direct Atomic Simulations of Facet
       | Formation and Equilibrium Shapes of SiC Nanoparticles"
       | 
       | Not as cool as experiment of course
       | 
       | https://pubs.acs.org/doi/full/10.1021/acs.cgd.9b00612
        
         | blix wrote:
         | This is a neat paper. Cool to see kinetic phenomena make it's
         | way into MD. How many GPU-hours did you need to get those 500ns
         | simulations?
         | 
         | You should throw up some videos of these somewhere, if you have
         | the time.
        
       | peter_d_sherman wrote:
       | _Star Trek 's Replicator -- version 0.000001..._ <g>
        
       | vhold wrote:
       | There are video files here :
       | https://pubs.acs.org/doi/10.1021/jacs.0c12100?goto=supportin...
        
       | fantod wrote:
       | This is super cool but who's idea was it to feature the video as
       | a pretty small gif on the side of the page?
        
         | codezero wrote:
         | literally every grad student in science fields - they don't
         | care about video compression or download quality - and gifs are
         | fast and easy to make and simple to grok and come out with
         | straightforward and predictable fidelity.
        
       | jasondclinton wrote:
       | Non-physicist question: why does the block of the forming crystal
       | move as a whole back and forth? Is this Brownian motion in
       | action?
        
         | magicalhippo wrote:
         | The containing structure (the carbon nanohorn as they call it),
         | is vibrating. So I'm guessing it's getting kicked around when
         | it touches the walls, so to speak.
        
         | hindsightbias wrote:
         | Guessing the crystals are probably connected in some lattice so
         | won't move independently. The expansion horizontally is gated
         | by the walls so it gets bounced around until it moves to a
         | wider section. There seems to be some ratio of horizontal vs
         | vertical growth.
        
       | jagraff wrote:
       | This is incredibly cool:
       | 
       | > Two novel techniques, atomic-resolution real-time video and
       | conical carbon nanotube confinement, allow researchers to view
       | never-before-seen details about crystal formation. The
       | observations confirm theoretical predictions about how salt
       | crystals form and could inform general theories about the way in
       | which crystal formation produces different ordered structures
       | from an otherwise disordered chemical mixture.
       | 
       | > To hold samples in place, we use atom-thick carbon nanohorns,
       | one of our previous inventions. With the stunning videos
       | Sakakibara captured, we immediately noticed the opportunity to
       | study the structural and statistical aspects of crystal
       | nucleation in unprecedented detail.
       | 
       | Creating shaped nucleation sites using carbon nanotubes
       | (nanohorns?) sounds like a fascinating technology. I don't have
       | access to the paper unfortunately - I'm curious what other types
       | of crystals could theoretically be grown with this technology.
       | The authors mention graphite - what about silicon? Could it be
       | used to grow more regular crystals for use in electronics? With
       | fewer defects, I'd imagine we could reduce the failure rate in
       | manufacturing.
        
         | grishka wrote:
         | > I don't have access to the paper unfortunately
         | 
         | The website you're looking for starts with sci and ends with
         | hub.
        
           | sebmellen wrote:
           | Not up there yet. Probably needs a few weeks, unless a HN
           | reader is so kind as to add it: https://sci-
           | hub.se/10.1021/jacs.0c12100.
        
           | Ericson2314 wrote:
           | Are you angling for some scintillating chub?
        
       | [deleted]
        
       | codercotton wrote:
       | Super cool, where's my replicator?
        
         | curtainsforus wrote:
         | Just build your own
        
       | [deleted]
        
       | thepace wrote:
       | Every time I see these kinds of video, whether that is of protein
       | translation, kinesin walking on microtubule, or birth and death
       | of a galaxy, I get this feeling that Panpsychism is closer to
       | truth that it gets credit for. Any constraints we put in the
       | defining consciousness and life seems to be just some arbitrary
       | constraint put there for our own convenience.
        
         | wahern wrote:
         | Panpsychism, pantheism, etc, are enticing because humans are
         | predisposed to see patterns, structure, reason, and
         | intelligence; to anthropomorphize nature. Characterizing as
         | "arbitrary" our admittedly feeble and flawed attempts at
         | distinguishing the human mind is an easy way to placate that
         | underlying, intrinsic desire.
         | 
         | Of course, maybe it is true! (That felt good to say :)
        
         | TeMPOraL wrote:
         | Isn't panpsychism a kind of reverse materialism? Both seem to
         | correctly recognize that terms we create are just lines we draw
         | on our map through the terrain of reality, which we rank by
         | their usefulness, by how close they seem to be "carving nature
         | at its joints". Based on my brief skimming, panpsychism seems
         | to say the terrain is all mysterious and wonderful, whereas
         | materialism says it's all just mundane.
         | 
         | Or am I completely mis-skimming the Wikipedia entry on
         | panpsychism?
        
           | perfmode wrote:
           | my question to you: do you consider yourself to be mysterious
           | or just mundane? what is your experience of your own Being-
           | ness?
        
             | TeMPOraL wrote:
             | A good question, something I'll have to think about.
             | 
             | The immediate if indirect answer I can give you: I stopped
             | feeling this sense of wonder, mystery, greater purpose of
             | reality, somewhen during my university years. I only ever
             | experience these feelings when consuming works of fiction.
        
           | lewispollard wrote:
           | I think you'd enjoy the work of Bernardo Kastrup, who is a
           | proponent of idealism, while also arguing against
           | panpsychism, for basically the reasons you just stated - ie,
           | there is a reality made of parts, and those parts are x,
           | where x is 'matter', 'mind', 'consciousness',
           | 'electromagnetism' and so on. But the trouble then is that
           | you can only describe the constituent parts in terms of those
           | parts. For example, subatomic particles have properties like
           | spin and charge, but that's the only way you can describe
           | them - in relation to one another - without having to go a
           | level 'deeper' if it were possible to describe them in
           | further parts (which would only be describable in terms of
           | those parts, and so on).
        
         | csomar wrote:
         | > Any constraints we put in the defining consciousness and life
         | seems to be just some arbitrary constraint put there for our
         | own convenience.
         | 
         | The definition of consciousness is very much tied to how humans
         | (or some scientists) perceive consciousness. I'm pretty sure my
         | dog is conscious of itself and its surrounding. It just happens
         | to have a less sophisticated consciousness than the one I have.
         | Some animals might have a pretty high consciousness but they
         | fail to communicate it to the humans.
        
         | kharak wrote:
         | I can't see this connection at all. Could someone who thinks or
         | feels this way elaborate?
         | 
         | Does this feeling arise because those atoms move? Or is it the
         | self-assembling behavior? Is this the same feeling some people
         | have when they see a door suddenly close due to the wind, as if
         | some spirit is responsible? I remember feeling like this as a
         | kid. But getting older, I realized that this feeling of agency
         | behind everything is unfounded. And the feeling faded away.
        
         | jes wrote:
         | I am an Alan Watts fan. I think he would agree with you.
        
           | djedr wrote:
           | He would definitely dig that. Curiously, I was drawn to this
           | thread because I was just listening to him today, talking
           | about crystals and the nature of reality. He would go thru so
           | many topics in such detail and clarity, it's incredible.
        
           | jng wrote:
           | I love Alan Watts too. In any case, I need to insert the
           | necessary reference to recently passed John Conway's Free
           | Will Theorem. I recommend every one to watch his 6-lecture
           | long presentation on this, available on YouTube and
           | underappreciated given the number of views, where he
           | captivatingly describes his proof that, if we have free will,
           | so do elementary particles. This is a purely mathematics- and
           | physics-based proof which I understand is fully accepted by
           | the scientific community, and while it, of course, does not
           | provide an explanation of the underlying cause, it provides
           | the best possible description obtained by scientific
           | methodology so far.
           | 
           | I like to think that, somehow, Alan Watts and John Conway
           | were digging the same tunnel, just starting from the two
           | endpoints, and bound to meet at some point in the future. We
           | just need a few more diggers of that stature (tall order, I
           | know).
        
       | [deleted]
        
       | jcims wrote:
       | I'm curious how they managed to make it happen so slowly. If that
       | crystal had grown to 100 molecules in 10 seconds it would take
       | roughly the age of the universe to form a grain of table salt.
        
         | jacquesm wrote:
         | The growth rate is proportional to the surface area.
        
         | goalieca wrote:
         | They confined the reaction to a tiny horn.
        
       | dragontamer wrote:
       | > "Salt is just our first model substance to probe the
       | fundamentals of nucleation events," said University Professor
       | Eiichi Nakamura. "Salt only crystallizes one way. But other
       | molecules, such as carbon, can crystallize in multiple ways,
       | leading to graphite or diamond. This is called polymorphism and
       | no one has seen the early stages of the nucleation that leads to
       | it. I hope our study provides the first step in understanding the
       | mechanism of polymorphism."
       | 
       | I'm amused that Chemists / Physicists also have the word
       | "Polymorphism" and that it means something completely different
       | from the programming term.
        
         | flobosg wrote:
         | It's also a term used in biology:
         | https://en.wikipedia.org/wiki/Polymorphism#Biology
        
         | skulk wrote:
         | My second confrontation with the term "polymorph" was a Java
         | tutorial, the first was Larn
         | (https://larn.fandom.com/wiki/Spells)
        
         | MereInterest wrote:
         | In some ways, they are sort of related. In chemistry, you have
         | different representations (diamond/graphite) of the same
         | underlying thing (carbon). In programming, you have different
         | representations (PointXY/PointRTheta) of the the same
         | underlying concept (Point2D).
        
           | jxramos wrote:
           | right, the roots of the word make it applicable to lots of
           | stuff, poly or many, morph or structure/form.
        
             | adrianmonk wrote:
             | Arguably it's the strategy pattern. Graphite and Diamond
             | are subclasses of CrystalizationStrategy.
        
       | soheil wrote:
       | This looks like how microscopic proteins and bacteria move in the
       | body. I wonder how much of their motion is caused by the atomic
       | level forces that form a lattice structure similar to that of
       | salt crystals.
        
         | rightbyte wrote:
         | The "tube"/horn is vibrating. I would make that connection from
         | the gif. The scale difference is quite big.
        
       | adrianmonk wrote:
       | Amazing achievement! Not only the world's first video of this
       | type, but I imagine also the world's smallest salt shaker.
        
       | [deleted]
        
       | frongpik wrote:
       | Another interesting experiment is the effect of strong magnetic
       | fields on crystals: when the field is turned off, is there
       | something left in the crystal, e.g. a certain motion pattern of
       | crystal nodes?
        
       | jerzyt wrote:
       | What is absolutely mind blowing to me is that when I was in
       | college, in my crystallography class, we were inferring the
       | crystal structure through the X-ray diffraction. Now we can
       | observe it directly. I took the crystallography class in late
       | 70s. I doubt that anyone had expected so much progress.
        
         | 6nf wrote:
         | In the same vein, I'm blown away what we can do with xray
         | crystallography these days! Structures of proteins with
         | hundreds of atoms can somehow be deduced from some tiny light
         | spots in a kaleidoscope picture? Magical.
        
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